北京大学学报(自然科学版)

基于物种间浓度相关法估算2012年中国HCFC-142b排放量

韩佳蕊1,李力1,方雪坤1,吴婧1,苏?1,温新元2,吴宇声1,胡建信1   

  1. 1. 区域环境质量协同创新中心, 环境模拟与污染控制国家重点联合实验室, 北京大学环境科学与工程学院, 北京 100871;2. 中山大学管理学院, 广州 510275;
  • 收稿日期:2013-08-19 出版日期:2015-01-20 发布日期:2015-01-20

Estimate of Anthropogenic HCFC-142b Emission from China in 2012 by Interspecies Correlation

HAN Jiarui1, LI Li1, FANG Xuekun1, WU Jing1, SU Shen1, WEN Xinyuan2, WU Yusheng1, HU Jianxin1   

  1. 1. Collaborative Innovation Center for Regional Environmental Quality, State Key Joint Laboratory of Environmental Simulation and Pollution Control, College of Environmental Sciences and Engineering, Peking University, Beijing 100871; 2. Sun Yat-Sen Business School, Sun Yat-Sen University, Guangzhou 510275;
  • Received:2013-08-19 Online:2015-01-20 Published:2015-01-20

摘要: 利用北京大学定点较高时间频率浓度监测数据, 甄选HCFC-22为估算HCFC-142b排放量适宜的参考物质, 分析认为以往基于背景地区数据的研究中普遍采用的参考物质CO不适用于利用城市地区大气样品进行物种间浓度相关法研究。根据全国四城市(北京、杭州、兰州和广州)四季的HCFC-142b及其参考物质浓度监测数据, 通过物种间浓度相关法计算2012年中国HCFC-142b排放量为16.24 (13.90~18.58) kt, 相当于1.06 ODP kt和37 Tg CO2-eq, 占2012年中国HCFCs 排放总量的9.78% (ODP), 占全球HCFC-142b排放总量的30.57%。中国HCFC-142b的减排淘汰工作将在未来中国和全球成功履约中占据重要地位。

关键词: 物种间浓度相关法, HCFC-142b, 排放清单, 臭氧消耗物质, 温室气体

Abstract: The high-time-resolution atmospheric mixing ratio data were sampled at Peking University. The data was analyzed and led to the conclusion that HCFC-22 was the proper reference substance; CO, the idiomatic reference, was not suitable for interspecies correlation analysis when dealing with data from urban districts. Based on the observation data of HCFC-142b and HCFC-22 gained from four representative cities (Beijing, Hangzhou, Lanzhou and Guangzhou) in four seasons, China’s HCFC-142b emission in 2012 was calculated by interspecies correlation. The result was 16.24 (13.90?18.58) kt, equivalent to 1.06 kt ODP and 37 Tg CO2-eq, taking up 9.78% (ODP) of total HCFCs emission in China or 30.5% of global HCFC-142b emission. Therefore, China’s HCFC-142b control would play an important role in phasing out HCFCs domestically and globally.

Key words: interspecies correlation, HCFC-142b, emission inventory, ozone depleting substance, greenhouse gas

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