3 MeV 金离子辐照Ni60Nb40 非晶合金及Hastelloy-N 合金的辐照损伤研究

doi:10.13209/j.0479-8023.2015.056

北京大学学报（自然科学版） ›› 2015, Vol. 51 ›› Issue (5): 783-790.DOI: 10.13209/j.0479-8023.2015.056

• 数学 • 下一篇

3 MeV 金离子辐照Ni₆₀Nb₄₀ 非晶合金及Hastelloy-N 合金的辐照损伤研究

刘士毅¹;徐光跃²;张艳文¹;王绪¹;唐美雄¹;赵子强¹;魏炳忱²

¹北京大学物理学院重离子物理国家重点实验室, 北京 100871;
²中国科学院力学研究所微重力国家重点实验室, 北京 100190;

收稿日期:2014-05-13 修回日期:2014-06-09 出版日期:2015-09-20 发布日期:2015-09-20
通讯作者: zqzhao@pku.edu.cn (赵子强); weibc@imech.ac.cn (魏炳忱)
基金资助:
国家自然科学基金(91226202)资助

Investigations on Irradiation Effects of Ni₆₀Nb₄₀ Amorphous Alloy and Hastelloy-N Alloy by 3 MeV Au Ion

LIU Shiyi¹;XU Guangyue²;ZHANG Yanwen¹;WANG Xu¹;TANG Meixiong¹;ZHAO Ziqiang¹;WEI Bingchen²

¹State Key Lab of Nuclear Physics and Technology, Peking University, Beijing 100871;
²Key Laboratory of Microgravity (National Microgravity Laboratory), Institute of Mechanics, Chinese Academy of Sciences, Beijing 100190;

Received:2014-05-13 Revised:2014-06-09 Online:2015-09-20 Published:2015-09-20
Contact: zqzhao@pku.edu.cn (ZHAO Ziqiang); weibc@imech.ac.cn (WEI Bingchen)

摘要/Abstract

摘要： 使用 3 MeV 金离子对Ni₆₀Nb₄₀ 非晶合金和Hastelloy-N 合金进行剂量为2.3×10¹⁵ cm^–2 和5×10¹⁶ cm^–2 的辐照实验。X 射线衍射(XRD)数据表明, Ni₆₀Nb₄₀ 非晶合金的非晶态在室温辐照下非常稳定, 而Hastelloy- N 合金在辐照后有明显的微观应变增加。同时纳米压痕分析表明, Ni₆₀Nb₄₀ 非晶合金的辐照软化和Hastelloy- N 合金的辐照硬化主要由原子移位损伤造成。使用原子力显微镜(AFM)测量半遮挡的辐照方法制造的肿胀台阶, 发现两种材料的辐照肿胀效应相差不大。扫描电子显微镜(SEM)观察发现, 室温条件下3 MeV 金离子导致Ni₆₀Nb₄₀ 非晶合金表面发生黏性流动的临界剂量大于2.3×10¹⁵ cm^–2, 而且发生线性流动的临界剂量具有不均匀性, 推测是由机械抛光时产生的表面应力造成。由于黏性流动可以有效修补表面缺陷, 所以Ni₆₀Nb₄₀ 非晶合金有希望作为抗腐蚀抗辐照涂层材料。

关键词: Hastelloy-N 合金, 镍基非晶合金, 熔盐反应堆, 辐照损伤, 黏性流动, 自修复

Abstract: 3 MeV Au ions were used to irradiate Hastelloy-N and Ni₆₀Nb₄₀ amorphous alloy, and total doses were 2.3×10¹⁵ cm^–2 and 5×10¹⁶ cm^–2. X-ray Diffraction results presented that Ni₆₀Nb₄₀ amorphous alloy showed good stability in crystal state, but Hastelloy-N had apparent strain increment after irradiation. Nano-Indenter test found that softening of Ni₆₀Nb₄₀ amorphous alloy and hardening of Hastelloy-N were mainly caused by atom displacement damage. Through measuring step heigh created by half-shielding irradiation with an Atomic Force Micoscope, the authors found that the irradiation swelling of both materials were approximate. Scan Electron Micoscope observation showed that the critical dose of Ni60Nb40 amorphous alloy surface viscous flow induced by 3 MeV Au ions was larger than 2.3×10¹⁵ cm^–2. The surface viscous flow critical dose was not uniform, which may be caused by surface stress induced by mechanical polishing. Ni₆₀Nb₄₀ amorphous alloy should be potential to be protective coating against corrosion and irradiation damage, for its self-healing of surface defects through viscous flow mechanism.

Key words: Hastelloy-N alloy, Ni-based amorphous alloy, molten salt reactor, irradiation damage, viscous flow, self-healing

刘士毅;徐光跃;张艳文;王绪;唐美雄;赵子强;魏炳忱. 3 MeV 金离子辐照Ni₆₀Nb₄₀ 非晶合金及Hastelloy-N 合金的辐照损伤研究[J]. 北京大学学报（自然科学版）, 2015, 51(5): 783-790.

LIU Shiyi;XU Guangyue;ZHANG Yanwen;WANG Xu;TANG Meixiong;ZHAO Ziqiang;WEI Bingchen. Investigations on Irradiation Effects of Ni₆₀Nb₄₀ Amorphous Alloy and Hastelloy-N Alloy by 3 MeV Au Ion[J]. Acta Scientiarum Naturalium Universitatis Pekinensis, 2015, 51(5): 783-790.

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https://xbna.pku.edu.cn/CN/Y2015/V51/I5/783

参考文献

[1] LeBlanc D. Molten salt reactors: a new beginning for an old idea. Nuclear Engineering and Design, 2010, 240(6): 1644–1656
[2] Mathieu L, Heuer D, Brissot R, et al. The thorium molten salt reactor: moving on from the MSBR. Progress in Nuclear Energy, 2006, 48(7): 664–679
[3] 林建波, 李爱国, 何上明. He+离子辐照后Hastelloy N 合金的耐腐蚀性研究. 核技术, 2014, 37(5): 050601
[4] Olson L C, Ambrosek J W, Sridharan K, et al. Materials corrosion in molten LiF-NaF-KF salt. Journal of Fluorine Chemistry, 2009, 130(1): 67–73
[5] Olson L C, Sridharan K, Anderson M, et al. Nickelplating for active metal dissolution resistance in molten fluoride salts. Journal of Nuclear Materials, 2011, 411: 51–59
[6] Liu Min, Lu Yanling, Liu Renduo, et al. TEM investigation on the microstructural evolution of hastelloy N induced by Ar+ ion irradiation. Micro北京大学学报(自然科学版) 第51 卷第 5 期 2015 年9 月 790 scopy Research and Technique, 2014, 77(2): 161–169
[7] Hunn J D, Lee E H, Byun T S, et al. Ion-irradiationinduced hardening in Inconel 718. J Nucl Mater, 2001, 296: 203–209
[8] Nagase T, Sanda T, Nino A, et al. MeV electron irradiation induced crystallization in metallic glasses: atomic structure, crystallization mechanism and stability of an amorphous phase under the irradiation. Journal of Non-Crystalline Solids, 2012, 358(3): 502– 518
[9] Hashimoto N, Hunn J D, Byun T S, et al. Microstructural analysis of ion-irradiation-induced hardening in inconel 718. J Nucl Mater, 2003, 318: 300–306
[10] Norgett M J, Robinson M T, Torrens I M. A proposed method of calculating displacement dose rates. Nucl Eng Des, 1975, 33(1): 50–54
[11] Audouard A, Balogh J, Dural J, et al. Displacement threshold energy of iron atoms in amorphous and crystalline Fe75B25 alloys. Radiation Effects and Defects in Solids, 1982, 62: 161–165
[12] Jin Shuoxue, Guo Liping, Yang Zheng, et al. Structural characterization of nickel-base alloy C-276 irradiated with Ar ions. Plasma Science and Technology, 2012, 14(6): 548–552
[13] Carter J, Fu E G, Martin M, et al. Effects of Cu ion irradiation in Cu50Zr45Ti5 metallic glass. Scripta Materialia, 2009, 61(3): 265–268
[14] Nagase T, Umakoshi Y. Temperature dependence in density-fluctuation-induced crystallization in metallic glass by MeV electron irradiation. Intermetallics, 2010, 18(10): 1803–1808
[15] Luo W D, Yang B, Chen G L. Effect of Ar+ ion irradiation on the microstructure and properties of Zr- Cu-Fe-Al bulk metallic glass. Scripta Materialia, 2011, 64(7): 625–628
[16] Trinkaus H, Ryazanov A I. Viscoelastic model for the plastic flow of amorphous solids under energetic ion bombardment. Phys Rev Lett, 1995, 74(25): 5072– 5075
[17] Gutzmann A, Klaumunzer S, Meier P. Ion-beaminduced surface instability of glassy Fe40Ni40B20. Phys Rev Lett, 1995, 74(12): 2256–2259

3 MeV 金离子辐照Ni₆₀Nb₄₀ 非晶合金及Hastelloy-N 合金的辐照损伤研究

Investigations on Irradiation Effects of Ni₆₀Nb₄₀ Amorphous Alloy and Hastelloy-N Alloy by 3 MeV Au Ion

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